Researchers led by Federico Capasso at Harvard John A. Paulson School of Engineering and Applied Sciences have developed methods to exert control over points of darkness, rather than light, using metasurfaces. “Dark regions in electromagnetic fields, or optical singularities, have traditionally posed a challenge due to their complex structures and the difficulty in shaping and sculpting them,” said Capasso, the Robert L. Wallace Professor of Applied Physics and Vinton Hayes Senior Research Fellow in Electrical Engineering at SEAS and senior corresponding author of two new papers describing the work. “These singularities, however, carry the potential for groundbreaking applications in fields such as remote sensing and precision measurement.” In 2011, Capasso’s lab introduced metasurfaces, or sub-wavelength-spaced arrays of nanostructures. In 2016, it used metasurfaces to build high-performance metalenses — flat optical lenses comprising nanopillars that they fabricated using semiconductor lithography techniques —which unlocked a new strategy to focus light using extremely lightweight devices. “Both of these studies introduce new classes of optical singularities — regions of designed darkness — using powerful but intuitive algorithms to inform the fabrication of metasurfaces,” said Soon Wei Daniel Lim, co-first author of the paper in Nature Communications with Joon-Suh Park. In that study, Lim and collaborators designed and fabricated an optical device containing metasurfaces of titanium dioxide nanopillars that can control light to create an array of optical singularities. To control exactly where these points of darkness appear, Lim used a computer algorithm to help him reverse engineer the design of the metasurface. Top: Scanning electron microscope image of the metasurface that generated the point singularities. Bottom: Experimental intensity profiles, with the point singularities labeled. Courtesy of Capasso Lab/Harvard SEAS. “I told the computer, here’s what I want to achieve in terms of dark spots; tell me what shape and diameter the nanopillars should be on this metasurface to make this happen,” Lim said. As light travels through the metasurface and lens, it generates a prescribed array of dark spots. “These dark spots are exciting because they could be used as optical traps to capture atoms,” Lim said. “It’s possible this could be used to simplify the optical architecture used in atomic physics labs, replacing today’s conventional equipment — instruments that take up 30 feet of space on a lab table — with compact, lightweight optical devices.” Dark spots aren’t just handy for trapping atoms. They can also be useful as highly precise reference positions for imaging. In its Science Advances paper, the Capasso group described a new class of optical singularities: extremely stable points of darkness in a polarized optical field, known as polarization singularities. “We've designed points of darkness that can withstand a wide range of perturbations — they are topologically protected,” said Christina Spaegele, first author of the paper. “This robustness opens the way to optical devices with high reliability and durability in various applications.” Previous research achieved some polarization singularities, but the conditions for maintaining that perfect spot of darkness were extremely fragile, making them easily destroyed by stray light or other environmental conditions. “By shining light through a specially designed metasurface and focusing lens, we can produce an unwavering polarization singularity surrounded entirely by points of light, essentially creating a dark spot inside a sphere of brightness,” Spaegele said. The technique is so robust that even introducing a defect to the metasurface doesn’t destroy the dark spot, but simply shifts its position. “This degree of control could be especially useful for imaging samples in ‘hostile’ environments, where vibrations, pressure, temperature, and stray light would typically interfere with imaging behavior,” Spaegele said. The team says these new developments in optical singularities have implications for remote sensing and covert detection. “Points of darkness could be used to mask out bright sources while imaging a scene, allowing us to see faint objects that are otherwise overshadowed,” Capasso said. “Objects or detectors placed at these dark positions will also not give away their position by scattering light, allowing them to be ‘hidden’ without affecting the surrounding light.” Harvard’s Office of Technology Development has protected the intellectual property arising from these studies and is exploring commercialization opportunities. The work was supported by the Air Force Office of Scientific Research and the European Research Council. The research was published in Nature Communications (www.doi.org/10.1038/s41467-023-39072-6) and Science Advances (www.doi.org/10.1126/sciadv.adh0369).