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Graphene Deploys as a Powerful Gas Sensor Emission Source

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Using graphene as the emission source, researchers at AMO GmbH worked with other European universities to develop a MIR emitter for integrated photonic gas sensors.

The researchers integrated the graphene-based emitter with photonic waveguides that couple directly into silicon waveguides operating in the region relevant for gas sensing. The integration of these components at the wafer level could reduce the size and cost, improve the mechanical stability, and potentially enhance the performance of environmental sensors.

Applications in environmental monitoring, industrial process control, medical diagnostics, and other areas require compact, reliable gas sensors to monitor air quality in real time. The graphene IR emitters, which could be used for a distributed network of sensors, offer a potential solution for gas sensor systems across various industries.

Traditional gas sensing methods are based on the chemical reaction of the targeted gas to the sensor material. The reaction of the gas affects the sensor, which can lead to the need for frequent calibration, drift, performance degradation, and a limited sensor lifetime.
A graphene-based infrared emitter for integrated photonic gas sensors. Courtesy of AMO GmbH.
A graphene-based IR emitter for integrated photonic gas sensors. Courtesy of AMO GmbH.

Absorption spectroscopy, in contrast, works by characterizing the absorption wavelengths of gases, such as greenhouse gases, and providing a spectral fingerprint that can be used to determine the composition of the gas. This method provides high specificity, minimal drift, and long-term stability without chemically altering the sensor. It is, therefore, useful for precise gas detection and robust, real-time air quality monitoring.

Photonic integrated circuits (PICs) can be used to shrink spectroscopy equipment to the size of a chip, creating a compact, cost-efficient optical gas sensor system. However, PIC-based gas sensors still require light coupling from external sources, and coupling to detectors in and out of the waveguides. Integrating light sources and detectors directly on the wafer could enable spectroscopic gas sensing in a highly compact format.

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The researchers chose to use graphene as the active material for their thermal MIR emitter because graphene can reach the temperatures necessary for thermal emission, and its emissivity is comparable to that of other very thin emitters. These properties make it a good source for MIR emission.

Monolayers of graphene are so thin that the entire emitting volume can be placed closest to the waveguide, generating ideal near-field coupling of the emission directly into the waveguide mode. Monolayer graphene causes minimal distortion to the waveguide mode, which lessens the mismatch between the mode in the emitter region and outside this region.

Researcher Nour Negm worked with colleagues at RWTH Aachen University, KTH Royal Institute of Technology, Senseair AB, and the University of Bundeswehr to integrate the graphene emitters on top of silicon photonic waveguides, enabling direct coupling of the emitters into the waveguide mode. The researchers operated the emitter for approximately one hour under ambient conditions, demonstrating MIR emission into the waveguide and out of a grating coupler. They detected emissions in the spectral range of 3 to 5 μm.

Based on thermal simulations, the researchers predict emitter temperatures could reach the range of 500 to 900 Kelvin, which is comparable with other nanoscale emitters. They estimate emission coupling efficiencies into the waveguide of up to 68%, which compares favorably with other nanoscale emitters.

Although the PIC used in the experiment was primarily characterized for a 4.2 μm wavelength targeting CO2 detection, the integrated graphene thermal emitters radiate in a broad gas absorption fingerprint wavelength range of 3 to 10 μm.

Combined with integrated graphene MIR photodetectors, the graphene MIR emitters could enable fully integrated photonic sensors, where the evanescent fields of the waveguides could interact directly with the gaseous environment, enabling their broad application for gas and environmental sensing.

The research was published in ACS Photonics (www.doi.org/10.1021/acsphotonics.3c01892).

Published: July 2024
Glossary
infrared
Infrared (IR) refers to the region of the electromagnetic spectrum with wavelengths longer than those of visible light, but shorter than those of microwaves. The infrared spectrum spans wavelengths roughly between 700 nanometers (nm) and 1 millimeter (mm). It is divided into three main subcategories: Near-infrared (NIR): Wavelengths from approximately 700 nm to 1.4 micrometers (µm). Near-infrared light is often used in telecommunications, as well as in various imaging and sensing...
graphene
Graphene is a two-dimensional allotrope of carbon consisting of a single layer of carbon atoms arranged in a hexagonal lattice pattern. It is the basic building block of other carbon-based materials such as graphite, carbon nanotubes, and fullerenes (e.g., buckyballs). Graphene has garnered significant attention due to its remarkable properties, making it one of the most studied materials in the field of nanotechnology. Key properties of graphene include: Two-dimensional structure:...
optoelectronics
Optoelectronics is a branch of electronics that focuses on the study and application of devices and systems that use light and its interactions with different materials. The term "optoelectronics" is a combination of "optics" and "electronics," reflecting the interdisciplinary nature of this field. Optoelectronic devices convert electrical signals into optical signals or vice versa, making them crucial in various technologies. Some key components and applications of optoelectronics include: ...
nano
An SI prefix meaning one billionth (10-9). Nano can also be used to indicate the study of atoms, molecules and other structures and particles on the nanometer scale. Nano-optics (also referred to as nanophotonics), for example, is the study of how light and light-matter interactions behave on the nanometer scale. See nanophotonics.
semiconductor
A semiconductor is a type of material that has electrical conductivity between that of a conductor and an insulator. In other words, semiconductors have properties that are intermediate between metals (good conductors of electricity) and insulators (poor conductors of electricity). The conductivity of a semiconductor can be controlled and modified by factors such as temperature, impurities, or an applied electric field. The most common semiconductors are crystalline solids, and they are...
integrated photonics
Integrated photonics is a field of study and technology that involves the integration of optical components, such as lasers, modulators, detectors, and waveguides, on a single chip or substrate. The goal of integrated photonics is to miniaturize and consolidate optical elements in a manner similar to the integration of electronic components on a microchip in traditional integrated circuits. Key aspects of integrated photonics include: Miniaturization: Integrated photonics aims to...
absorption spectroscopy
Absorption spectroscopy is a fundamental analytical technique used to study the interaction between electromagnetic radiation and matter. It involves measuring the absorption of light by a sample across a range of wavelengths or frequencies. This absorption is caused by the sample's ability to absorb certain wavelengths of light, which corresponds to the excitation of electrons or molecules to higher energy levels. Principle of absorption: Absorption occurs when the energy of incident...
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